Charlotte, North Carolina is 3.5 times larger than Baltimore.
Area: 212 km2 calculated
Baltimore is the largest city in the U.S. state of Maryland and the 26th-most populous city in the country. It is located in the central area of the state along the tidal portion of the Patapsco River, an arm of the Chesapeake Bay. Wikipedia
Area: 733 km2 calculated
Charlotte is the largest city in the U.S. state of North Carolina and the seat of Mecklenburg County. In 2013, the estimated population of Charlotte according to the U.S. Census Bureau was 792,862, making it the 16th largest city in the United States based on population. Wikipedia